EMSL Magnetic Resonance Users Quantify Radiation Damage in
Actinide Waste Containment Material. Users of the William R. Wiley
Environmental Molecular Sciences Laboratory (EMSL) have improved the
fundamental understanding and predictive models that support the informative
evaluation of the long-term stability of materials proposed for immobilization
of actinide wastes. Scientists from the University of Cambridge and Pacific Northwest National
Laboratory (PNNL) presented research in an article in this week’s Nature
(Vol 445, pg 190-193) that analyzes the impacts of
alpha-emitters on the crystalline structure of zircon. These results measured
significantly more atoms displaced by each alpha-disintegration in zircon than
had previously been estimated. The
authors were also able to show that damage in synthetic plutonium-doped zircon
samples is likely to be consistent with damage resulting from long-term,
lower-level exposure experienced by naturally occurring, uranium-containing
zircons. Portions of this research were
conducted using the EMSL, a DOE national scientific user facility at PNNL. EMSL scientists collaborated on the
development of triple containment rotor technology and provided user access for
the radiological nuclear magnetic resonance magic-angle spinning analysis. This
publication highlights how EMSL’s unique capabilities
attract international users and collaborators and promote high-impact science.